Fluoride removal from waters by Donnan dialysis
Identifieur interne : 000D62 ( Main/Exploration ); précédent : 000D61; suivant : 000D63Fluoride removal from waters by Donnan dialysis
Auteurs : Mustapha Hichour [France] ; Françoise Persin [France] ; Jacqueline Sandeaux [France] ; Claude Gavach [France]Source :
- Separation and Purification Technology [ 1383-5866 ] ; 1999.
Abstract
Excess or lack of levels of fluoride in drinking water being harmful to human health, the concentration of F− ions must be maintained in the range 0.5 to 1.5mgl−1. The purpose of this study is to apply Donnan dialysis (DD) for fluoride removal from waters with a concentration exceeding the permitted value. Two synthetic waters, which are models of waters from countries of Africa (Maghreb, Senegal), were prepared and treated with a DD pre-industrial pilot. The anion exchange membrane was the DSV membrane (Asahi Glass), with a total area of 0.176m2. The initial fluoride concentration was 9.5 and 6.1mgl−1 in each model water, respectively. The DD process was studied under two circulating modes of the receiver solution, single pass and batch, while the feed solution flowed continuously as a single pass. To maintain the fluoride concentration below the acceptable values at the outlet of the feed compartment, the extracted fluoride ions are complexed by Al3+ ions which were added in the receiver solution. Chemical speciation of aluminum–fluoride compounds was studied in order to define the optimized conditions of pH and concentration. Despite the different anions (Cl−, HCO−3, SO2−4) and cations (Na+, K+, Ca2+, Mg2+) generally present in ground waters, a fluoride concentration in agreement with the norm (<1.5mgl−1) could be reached whatever the water treated. However, the mineralization of water was increased by about 25% resulting from the electrolyte diffusion which occurs from the receiver to the feed solution.
Url:
DOI: 10.1016/S1383-5866(99)00042-8
Affiliations:
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The purpose of this study is to apply Donnan dialysis (DD) for fluoride removal from waters with a concentration exceeding the permitted value. Two synthetic waters, which are models of waters from countries of Africa (Maghreb, Senegal), were prepared and treated with a DD pre-industrial pilot. The anion exchange membrane was the DSV membrane (Asahi Glass), with a total area of 0.176m2. The initial fluoride concentration was 9.5 and 6.1mgl−1 in each model water, respectively. The DD process was studied under two circulating modes of the receiver solution, single pass and batch, while the feed solution flowed continuously as a single pass. To maintain the fluoride concentration below the acceptable values at the outlet of the feed compartment, the extracted fluoride ions are complexed by Al3+ ions which were added in the receiver solution. Chemical speciation of aluminum–fluoride compounds was studied in order to define the optimized conditions of pH and concentration. Despite the different anions (Cl−, HCO−3, SO2−4) and cations (Na+, K+, Ca2+, Mg2+) generally present in ground waters, a fluoride concentration in agreement with the norm (<1.5mgl−1) could be reached whatever the water treated. However, the mineralization of water was increased by about 25% resulting from the electrolyte diffusion which occurs from the receiver to the feed solution.</div></front></TEI><affiliations><list><country><li>France</li></country><region><li>Languedoc-Roussillon</li><li>Occitanie (région administrative)</li></region><settlement><li>Montpellier</li></settlement></list><tree><country name="France"><region name="Occitanie (région administrative)"><name sortKey="Hichour, Mustapha" sort="Hichour, Mustapha" uniqKey="Hichour M" first="Mustapha" last="Hichour">Mustapha Hichour</name></region><name sortKey="Gavach, Claude" sort="Gavach, Claude" uniqKey="Gavach C" first="Claude" last="Gavach">Claude Gavach</name><name sortKey="Persin, Francoise" sort="Persin, Francoise" uniqKey="Persin F" first="Françoise" last="Persin">Françoise Persin</name><name sortKey="Sandeaux, Jacqueline" sort="Sandeaux, Jacqueline" uniqKey="Sandeaux J" first="Jacqueline" last="Sandeaux">Jacqueline Sandeaux</name><name sortKey="Sandeaux, Jacqueline" sort="Sandeaux, Jacqueline" uniqKey="Sandeaux J" first="Jacqueline" last="Sandeaux">Jacqueline Sandeaux</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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